From The Collaborative International Dictionary of English v.0.44 [gcide]:
Attune \At*tune"\, verb (used with an object) [imp. & p. p. {Attuned}; p. pr. & vb. n. {Attuning}.] [Pref. ad- + tune.]
1. To tune or put in tune; to make melodious; to adjust, as one sound or musical instrument to another; as, to attune the voice to a harp.
2. To arrange fitly; to make accordant.
Wake to energy each social aim, Attuned spontaneous to the will of Jove. --Beattie.
From WordNet (r) 2.0 [wn]:
verb
1: adjust or accustom to; bring into harmony with
From Moby Thesaurus II by Grady Ward, 1.0 [moby-thes]:
67 Moby Thesaurus words for "attune": accommodate, accord, adapt, adjust, adjust to, agree, assimilate, assonate, atone, balance, be harmonious, be in tune, blend, capacitate, chime, chord, compensate, condition, conform, coordinate, counterbalance, cut to, enable, equalize, equip, fit, fix, furnish, gear to, harmonize, homologate, homologize, integrate, key to, make plumb, make uniform, measure, melodize, musicalize, proportion, put in trim, put in tune, qualify, reconcile, rectify, regulate, right, set, set right, set to rights, similarize, sound in tune, sound together, string, suit, symphonize, sync, synchronize, tailor, tone down, tone up, trim to, true, true up, tune, tune up, voice
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